Enhanced Ultraviolet Stability of Air-Processed Polymer Solar Cells by Al Doping of the ZnO Interlayer.
Identifieur interne : 001F88 ( Main/Exploration ); précédent : 001F87; suivant : 001F89Enhanced Ultraviolet Stability of Air-Processed Polymer Solar Cells by Al Doping of the ZnO Interlayer.
Auteurs : Mario Prosa [Italie] ; Marta Tessarolo [Italie] ; Margherita Bolognesi [Italie] ; Olivier Margeat [France] ; Desta Gedefaw [Suède] ; Meriem Gaceur [France] ; Christine Videlot-Ackermann [France] ; Mats R. Andersson [Suède] ; Michele Muccini [Italie] ; Mirko Seri [Italie] ; Jörg Ackermann [France]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2016.
Abstract
Photostability of organic photovoltaic devices represents a key requirement for the commercialization of this technology. In this field, ZnO is one of the most attractive materials employed as an electron transport layer, and the investigation of its photostability is of particular interest. Indeed, oxygen is known to chemisorb on ZnO and can be released upon UV illumination. Therefore, a deep analysis of the UV/oxygen effects on working devices is relevant for the industrial production where the coating processes take place in air and oxygen/ZnO contact cannot be avoided. Here we investigate the light-soaking stability of inverted organic solar cells in which four different solution-processed ZnO-based nanoparticles were used as electron transport layers: (i) pristine ZnO, (ii) 0.03 at %, (iii) 0.37 at %, and (iv) 0.8 at % aluminum-doped AZO nanoparticles. The degradation of solar cells under prolonged illumination (40 h under 1 sun), in which the ZnO/AZO layers were processed in air or inert atmosphere, is studied. We demonstrate that the presence of oxygen during the ZnO/AZO processing is crucial for the photostability of the resulting solar cell. While devices based on undoped ZnO were particularly affected by degradation, we found that using AZO nanoparticles the losses in performance, due to the presence of oxygen, were partially or totally prevented depending on the Al doping level.
DOI: 10.1021/acsami.5b08255
PubMed: 26751271
Affiliations:
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Gobetti, 101, 40129 Bologna, Italy.</nlm:affiliation><country xml:lang="fr">Italie</country><wicri:regionArea>Consiglio Nazionale delle Ricerche (CNR) - Istituto per lo Studio dei Materiali Nanostrutturati (ISMN) , Via P. Gobetti, 101, 40129 Bologna</wicri:regionArea><wicri:noRegion>40129 Bologna</wicri:noRegion></affiliation></author><author><name sortKey="Tessarolo, Marta" sort="Tessarolo, Marta" uniqKey="Tessarolo M" first="Marta" last="Tessarolo">Marta Tessarolo</name><affiliation wicri:level="1"><nlm:affiliation>Consiglio Nazionale delle Ricerche (CNR) - Istituto per lo Studio dei Materiali Nanostrutturati (ISMN) , Via P. Gobetti, 101, 40129 Bologna, Italy.</nlm:affiliation><country xml:lang="fr">Italie</country><wicri:regionArea>Consiglio Nazionale delle Ricerche (CNR) - Istituto per lo Studio dei Materiali Nanostrutturati (ISMN) , Via P. Gobetti, 101, 40129 Bologna</wicri:regionArea><wicri:noRegion>40129 Bologna</wicri:noRegion></affiliation></author><author><name sortKey="Bolognesi, Margherita" sort="Bolognesi, Margherita" uniqKey="Bolognesi M" first="Margherita" last="Bolognesi">Margherita Bolognesi</name><affiliation wicri:level="1"><nlm:affiliation>Laboratory MIST E-R , Via P. Gobetti, 101, 40129 Bologna, Italy.</nlm:affiliation><country xml:lang="fr">Italie</country><wicri:regionArea>Laboratory MIST E-R , Via P. Gobetti, 101, 40129 Bologna</wicri:regionArea><wicri:noRegion>40129 Bologna</wicri:noRegion></affiliation></author><author><name sortKey="Margeat, Olivier" sort="Margeat, Olivier" uniqKey="Margeat O" first="Olivier" last="Margeat">Olivier Margeat</name><affiliation wicri:level="4"><nlm:affiliation>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille</wicri:regionArea><wicri:noRegion>13288 Marseille</wicri:noRegion><placeName><settlement type="city">Marseille</settlement><region type="région" nuts="2">Provence-Alpes-Côte d'Azur</region><settlement type="city">Marseille</settlement></placeName><orgName type="university">Université d'Aix-Marseille</orgName></affiliation></author><author><name sortKey="Gedefaw, Desta" sort="Gedefaw, Desta" uniqKey="Gedefaw D" first="Desta" last="Gedefaw">Desta Gedefaw</name><affiliation wicri:level="1"><nlm:affiliation>Department of Chemistry and Chemical Engineering, Polymer Technology, Chalmers University of Technology , Goteborg SE-412 96, Sweden.</nlm:affiliation><country xml:lang="fr">Suède</country><wicri:regionArea>Department of Chemistry and Chemical Engineering, Polymer Technology, Chalmers University of Technology , Goteborg SE-412 96</wicri:regionArea><wicri:noRegion>Goteborg SE-412 96</wicri:noRegion></affiliation></author><author><name sortKey="Gaceur, Meriem" sort="Gaceur, Meriem" uniqKey="Gaceur M" first="Meriem" last="Gaceur">Meriem Gaceur</name><affiliation wicri:level="4"><nlm:affiliation>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille</wicri:regionArea><wicri:noRegion>13288 Marseille</wicri:noRegion><placeName><settlement type="city">Marseille</settlement><region type="région" nuts="2">Provence-Alpes-Côte d'Azur</region><settlement type="city">Marseille</settlement></placeName><orgName type="university">Université d'Aix-Marseille</orgName></affiliation></author><author><name sortKey="Videlot Ackermann, Christine" sort="Videlot Ackermann, Christine" uniqKey="Videlot Ackermann C" first="Christine" last="Videlot-Ackermann">Christine Videlot-Ackermann</name><affiliation wicri:level="4"><nlm:affiliation>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille</wicri:regionArea><wicri:noRegion>13288 Marseille</wicri:noRegion><placeName><settlement type="city">Marseille</settlement><region type="région" nuts="2">Provence-Alpes-Côte d'Azur</region><settlement type="city">Marseille</settlement></placeName><orgName type="university">Université d'Aix-Marseille</orgName></affiliation></author><author><name sortKey="Andersson, Mats R" sort="Andersson, Mats R" uniqKey="Andersson M" first="Mats R" last="Andersson">Mats R. Andersson</name><affiliation wicri:level="1"><nlm:affiliation>Department of Chemistry and Chemical Engineering, Polymer Technology, Chalmers University of Technology , Goteborg SE-412 96, Sweden.</nlm:affiliation><country xml:lang="fr">Suède</country><wicri:regionArea>Department of Chemistry and Chemical Engineering, Polymer Technology, Chalmers University of Technology , Goteborg SE-412 96</wicri:regionArea><wicri:noRegion>Goteborg SE-412 96</wicri:noRegion></affiliation></author><author><name sortKey="Muccini, Michele" sort="Muccini, Michele" uniqKey="Muccini M" first="Michele" last="Muccini">Michele Muccini</name><affiliation wicri:level="1"><nlm:affiliation>Consiglio Nazionale delle Ricerche (CNR) - Istituto per lo Studio dei Materiali Nanostrutturati (ISMN) , Via P. Gobetti, 101, 40129 Bologna, Italy.</nlm:affiliation><country xml:lang="fr">Italie</country><wicri:regionArea>Consiglio Nazionale delle Ricerche (CNR) - Istituto per lo Studio dei Materiali Nanostrutturati (ISMN) , Via P. Gobetti, 101, 40129 Bologna</wicri:regionArea><wicri:noRegion>40129 Bologna</wicri:noRegion></affiliation></author><author><name sortKey="Seri, Mirko" sort="Seri, Mirko" uniqKey="Seri M" first="Mirko" last="Seri">Mirko Seri</name><affiliation wicri:level="1"><nlm:affiliation>Consiglio Nazionale delle Ricerche (CNR) - Istituto per la Sintesi Organica e la Fotoreattività (ISOF) , Via P. Gobetti, 101, 40129 Bologna, Italy.</nlm:affiliation><country xml:lang="fr">Italie</country><wicri:regionArea>Consiglio Nazionale delle Ricerche (CNR) - Istituto per la Sintesi Organica e la Fotoreattività (ISOF) , Via P. Gobetti, 101, 40129 Bologna</wicri:regionArea><wicri:noRegion>40129 Bologna</wicri:noRegion></affiliation></author><author><name sortKey="Ackermann, Jorg" sort="Ackermann, Jorg" uniqKey="Ackermann J" first="Jörg" last="Ackermann">Jörg Ackermann</name><affiliation wicri:level="4"><nlm:affiliation>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Aix-Marseille Université, CNRS , CINaM UMR 7325, 13288 Marseille</wicri:regionArea><wicri:noRegion>13288 Marseille</wicri:noRegion><placeName><settlement type="city">Marseille</settlement><region type="région" nuts="2">Provence-Alpes-Côte d'Azur</region><settlement type="city">Marseille</settlement></placeName><orgName type="university">Université d'Aix-Marseille</orgName></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Photostability of organic photovoltaic devices represents a key requirement for the commercialization of this technology. In this field, ZnO is one of the most attractive materials employed as an electron transport layer, and the investigation of its photostability is of particular interest. Indeed, oxygen is known to chemisorb on ZnO and can be released upon UV illumination. Therefore, a deep analysis of the UV/oxygen effects on working devices is relevant for the industrial production where the coating processes take place in air and oxygen/ZnO contact cannot be avoided. Here we investigate the light-soaking stability of inverted organic solar cells in which four different solution-processed ZnO-based nanoparticles were used as electron transport layers: (i) pristine ZnO, (ii) 0.03 at %, (iii) 0.37 at %, and (iv) 0.8 at % aluminum-doped AZO nanoparticles. The degradation of solar cells under prolonged illumination (40 h under 1 sun), in which the ZnO/AZO layers were processed in air or inert atmosphere, is studied. We demonstrate that the presence of oxygen during the ZnO/AZO processing is crucial for the photostability of the resulting solar cell. While devices based on undoped ZnO were particularly affected by degradation, we found that using AZO nanoparticles the losses in performance, due to the presence of oxygen, were partially or totally prevented depending on the Al doping level.</div></front></TEI><affiliations><list><country><li>France</li><li>Italie</li><li>Suède</li></country><region><li>Provence-Alpes-Côte d'Azur</li></region><settlement><li>Marseille</li></settlement><orgName><li>Université d'Aix-Marseille</li></orgName></list><tree><country name="Italie"><noRegion><name sortKey="Prosa, Mario" sort="Prosa, Mario" uniqKey="Prosa M" first="Mario" last="Prosa">Mario Prosa</name></noRegion><name sortKey="Bolognesi, Margherita" sort="Bolognesi, Margherita" uniqKey="Bolognesi M" first="Margherita" last="Bolognesi">Margherita Bolognesi</name><name sortKey="Muccini, Michele" sort="Muccini, Michele" uniqKey="Muccini M" first="Michele" last="Muccini">Michele Muccini</name><name sortKey="Seri, Mirko" sort="Seri, Mirko" uniqKey="Seri M" first="Mirko" last="Seri">Mirko Seri</name><name sortKey="Tessarolo, Marta" sort="Tessarolo, Marta" uniqKey="Tessarolo M" first="Marta" last="Tessarolo">Marta Tessarolo</name></country><country name="France"><region name="Provence-Alpes-Côte d'Azur"><name sortKey="Margeat, Olivier" sort="Margeat, Olivier" uniqKey="Margeat O" first="Olivier" last="Margeat">Olivier Margeat</name></region><name sortKey="Ackermann, Jorg" sort="Ackermann, Jorg" uniqKey="Ackermann J" first="Jörg" last="Ackermann">Jörg Ackermann</name><name sortKey="Gaceur, Meriem" sort="Gaceur, Meriem" uniqKey="Gaceur M" first="Meriem" last="Gaceur">Meriem Gaceur</name><name sortKey="Videlot Ackermann, Christine" sort="Videlot Ackermann, Christine" uniqKey="Videlot Ackermann C" first="Christine" last="Videlot-Ackermann">Christine Videlot-Ackermann</name></country><country name="Suède"><noRegion><name sortKey="Gedefaw, Desta" sort="Gedefaw, Desta" uniqKey="Gedefaw D" first="Desta" last="Gedefaw">Desta Gedefaw</name></noRegion><name sortKey="Andersson, Mats R" sort="Andersson, Mats R" uniqKey="Andersson M" first="Mats R" last="Andersson">Mats R. 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